SAMPE Journal - January/February 2022 - 28

FEATURE / RAPID CURING EPOXY
Figure 6. DMTA measurements representing
G'(blue), G " (green), and tan delta (red) as a
function of temperature.
Figure 7. Effect of cure schedule during HP-RTM on the
degree of cure attained by the composite panels. The
degree of cure determined via DMTA measurements
are shown as the blue symbols while the model
calculations are shown as the dashed lines.
to be a simple and efficient approach to capture
the relative change in the degree of cure for various
processing conditions employed in this work.
Other approaches for assessment
of cure levels
such as the use of DSC would be less effective for
these composite panels due to the complications
involved in separation of heat flow contributions
from the fiber fractions and the challenges or
uncertainties involved in analysis of residual cure
exotherms of very low magnitude. The panel cured
for 4 minutes at 115°C, shows a high Tg of 134°C
based on the tan delta peak method. The ultimate
Tg for the panels was found to be 141 ± 1.8°C based
on a second DMTA second for seven samples.
Hence, based on Equation 1, the experimental
results from the composite panels confirm the
potential to achieve 95% cure even for a very short
cure duration of 4 minutes, a nominal temperature
of 115°C.
The values of the experimentally determined
degree of cure determined from Equation 1
for panels produced under various processing
histories are compared with the model predictions
for the same thermal histories in Figure 7. The
degree of cure estimated from characterization
of the composite panels are found to be in close
agreement with the model predictions over the
entire range of processing conditions employed
in this work, which confirms and validates the fast
reactivity of the epoxy system developed in this
work. The degree of cure is found to be 95% at cure
temperatures of 110-115°C over the short durations
employed in this work. The results also show that
the degree of cure may vary over a range of 87-95%,
depending on the choice of cure temperature and
time in this work. The impact of these variations in
the degree of cure on the mechanical properties of
the composite panels will be explored in detail in
the subsequent section.
The effect of variation in the degree of cure
28 | SAMPE JOURNAL | JANUARY/FEBRUARY 2022
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SAMPE Journal - January/February 2022

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