SAMPE Journal - July/August 2022 - 61

Resin
Storage
Modules
(MPa)
With GY285
3a5610
35700
35900
5292B-PPA
BisA-PPA
BisM-PPA
5292B-FA
BisA-FA
BisF-FA
Thio-FA
With MY0610
35610
35700
35900
5292B-PPA
BisA-PPA
BisM-PPA
5292B-FA
BisA-FA
BisF-FA
Thio-FA
3086
2937
3763
3374
3349
3131
3162
3538
3433
3202
E' onset Tg
(o
C)
134
130
141
147
189
155
113
131
132
134
Loss Modulus
Peak (o
C)
148
149
154
171
203
170
137
155
157
157
Tan δ Peak
(o
C)
158
164
166
191
229
200
163
188
191
190
5% Weight
Loss
(o
C, in N2
360
362
346
309
304
357
340
345
341
)
Char Yield
at 800o
(%, in N2
31
41
39
31
30
36
41
49
48
C
)
2865
3322
3715
3444
3488
3359
3574
3834
3493
3058
220
214
225
221
239
225
204
221
221
216
240
231
233
236
247
234
207
234
226
232
Table 4. Curing result of benzoxazine and epoxy.
Thermal stability was reduced in most case as
expected. The reduction of char yield percentage
of the co-polymer with epoxy resin is reduce by
around 10 points. The decreasing of 5% weight loss
temperature in nitrogen varies wildly, from almost
no change for aniline benzoxazine/GY285 to oven
100°C different with Propargylamine/610 mixture.
Even though, those furfuryl amine benzoxazine
mixture still better than the aniline benzoxazine
mixture or propargylamine benzoxazine/epoxy
mixture.
Co-Polymerization of Benzoxazine and
Matrimid 5292A
Matrimid 5292A is the bismaleimide manufactured
by Huntsman Corporation. It has been used for
very high temperature composition in aerospace
industry. It has a melting point about 159°C, and
DSC scan at 10°C/min indicate its exotherm peak
at 273°C. The blend with benzoxazine often boost
the Tg and thermal stability. In our initial test, for
www. sampe.org
260
254
261
259
268
245
236
257
253
257
348
349
343
321
303
298
343
334
339
333
33
37
39
32(750o
34
36
39
41
47
48
C)
Figure 3. DSC of benzoxazine and BMI.
JULY AUGUST 2022
|
SAMPE JOURNAL |
61
http://www.sampe.org

SAMPE Journal - July/August 2022

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